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Royal Society of Chemistry, Chemical Society Reviews, 5(45), p. 1197-1210, 2016
DOI: 10.1039/c5cs00566c
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To rebound or dissociate? This is the mechanistic question in C–H hydroxylation by heme and nonheme metal–oxo complexes
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Abstract
Metal–oxo species can perform hydroxylation reactions via the rebound mechanism, but this review focuses on the cases where dissociative non-rebound mechanism is shown to dominate, with an emphasis on theoretical calculations.