Published in
Royal Society of Chemistry, Faraday Discussions, (194), p. 305-324
DOI: 10.1039/c6fd00103c
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Stimulated x-ray Raman Scattering – a critical assessment of the building block of nonlinear x-ray spectroscopy
,
Laurent Mercadier,
Clemens Weninger,
Alberto Lutman,
Daniel Ratner,
Ryan N. Coffee,
Maximilian Bucher,
Conny Såthe,
Christoph Bostedt,
Melanie Mucke,
Marcus Agåker,
Joseph Nordgren,
Jan-Erik Rubensson,
Nina Rohringer
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Abstract
SeriesInformation ; Faraday discussions 194, 305 - 324(2016). doi:10.1039/C6FD00103C ; Abstract ; With the invention of femtosecond X-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics reach a new era, allowing for time-resolved X-ray diffraction and spectroscopy. To ultimately probe coherent electron and nuclear dynamics on their natural time and length scales, coherent nonlinear X-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realisation of nonlinear X-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated resonant X-ray Raman scattering in molecular gas targets. ; Other ; Published by Soc., Cambridge [u.a.]