Published in
Royal Society of Chemistry, Chemical Communications, 32(52), p. 5585-5588, 2016
DOI: 10.1039/c6cc01368f
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Crystalline-like structures and multilayering in Langmuir films of ionic liquids at the air–water interface
Journal article published in 2016 by
Eduardo J. M. Filipe,
Pedro Morgado,
Miguel Teixeira,
Karina Shimizu 
,
Nathalie Bonatout,
Michel Goldmann,
José Nuno Canongia Lopes ,
José Nuno Canongia Lopes
,
Nathalie Bonatout,
Michel Goldmann,
José Nuno Canongia Lopes ,
José Nuno Canongia Lopes
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Abstract
Langmuir films of [C18mim][NTf2] ionic liquid exhibited, for the first time, the reversible formation of crystalline-like structures at the surface of water, compatible with the formation of multilayers. Atomistic molecular dynamics simulation results support the experimental findings, unambiguously indicating the existence of a trilayer.