Published in
Royal Society of Chemistry, Chemical Communications, 5(48), p. 663-665
DOI: 10.1039/c1cc16580a
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Redox mediation enabled by immobilised centres in the pores of a metal-organic framework grown by liquid phase epitaxy
Journal article published in 2012 by
André Dragässer,
Osama Shekhah,
Olexandra Zybaylo,
Cai Shen,
Manfred Buck,
Christof Wöll,
Derck Schlettwein 
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Abstract
A layer of a metal-organic framework (SURMOF) was prepared on a thiol monolayer on Au. Charge transport across the insulating membrane could be established by using ferrocene as an immobilised redox mediator. Reversibility of the immobilisation and its role in the electrode kinetics are discussed.