Published in
Royal Society of Chemistry, Chemical Communications, 25(47), p. 7158
DOI: 10.1039/c0cc05360k
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Fluctuations of the Stokes and anti-Stokes surface-enhanced resonance Raman scattering intensities in an electrochemical environment
Journal article published in 2011 by
Diego P. dos Santos,
Gustavo F. S. Andrade,
Alexandre G. Brolo,
Marcia L. A. Temperini 
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Abstract
Stokes and anti-Stokes SERRS intensity fluctuations were observed from a roughened silver electrode immersed in diluted solutions of Brilliant Green (BG), a behaviour linked to single-molecule events. The distributions of the anti-Stokes to Stokes ratios were obtained and their shape showed a strong dependence on the applied potential.