Published in
Royal Society of Chemistry, Organic Chemistry Frontiers, 3(11), p. 673-683, 2024
DOI: 10.1039/d3qo01779f
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N-heterocyclic nitrenium charge transfer catalysis via inner-sphere electron transfer in concert with halogen-atom dissociation
Journal article published in 2024 by
Chao-Shen Zhang,
Chang-Zhen Fang,
Liang Yi,
Chen Zhu 
,
Zhi-Xiang Wang ,
Xiang-Yu Chen ,
Magnus Rueping
,
Zhi-Xiang Wang ,
Xiang-Yu Chen ,
Magnus Rueping
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Abstract
We report an efficient and versatile catalytic N-heterocyclic nitrenium charge transfer complex strategy for the single-electron reduction of chloroform, resulting in the generation of the dichloromethyl radical for use in various transformations.