Published in
Royal Society of Chemistry, Energy & Environmental Science, 2024
DOI: 10.1039/d3ee04235a
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Operando investigations of the solid electrolyte interphase in the lithium mediated nitrogen reduction reaction
Journal article published in 2024 by
Niklas H. Deissler 
,
J. Bjarke V. Mygind ,
Katja Li ,
Valerie A. Niemann ,
Peter Benedek ,
Valentin Vinci,
Shaofeng Li,
Xianbiao Fu,
Peter C. K. Vesborg ,
Thomas F. Jaramillo ,
Jakob Kibsgaard ,
Jakub Drnec,
Ib Chorkendorff
,
J. Bjarke V. Mygind ,
Katja Li ,
Valerie A. Niemann ,
Peter Benedek ,
Valentin Vinci,
Shaofeng Li,
Xianbiao Fu,
Peter C. K. Vesborg ,
Thomas F. Jaramillo ,
Jakob Kibsgaard ,
Jakub Drnec,
Ib Chorkendorff
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Abstract
Operando GI-WAXS showed that the SEI layer formed by LiBF4 enhances Li-NRR performance by limiting proton transport to the electrode. Intermediate LiNxHy species give insight into the mechanism of Li-NRR.