Published in
Royal Society of Chemistry, Dalton Transactions, 18(52), p. 5918-5925, 2023
DOI: 10.1039/d3dt00299c
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An investigation into the Brønsted acidity of the perfluorinated alkoxy silanes {(F<sub>3</sub>C)<sub>3</sub>CO}<sub>3</sub>SiH and {(F<sub>6</sub>C<sub>5</sub>)<sub>3</sub>CO}<sub>2</sub>Si(Cl)H
Journal article published in 2023 by
Felix Feige,
Lorraine A. Malaspina,
Florian Kleemiss 
,
Julius F. Kögel,
Sergey Ketkov ,
Emanuel Hupf,
Simon Grabowsky ,
Jens Beckmann
,
Julius F. Kögel,
Sergey Ketkov ,
Emanuel Hupf,
Simon Grabowsky ,
Jens Beckmann
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Abstract
The Si–H bond in {(F3C)3CO}3SiH is exceptionally strong and short; yet the acidity is comparable to common organic acids. This apparent contradiction will be discussed with the aid of contemporary DFT methods.