Published in
Royal Society of Chemistry, Physical Chemistry Chemical Physics, 4(24), p. 2318-2331, 2022
DOI: 10.1039/d1cp04316a
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From graphene to graphene oxide: the importance of extended topological defects
Journal article published in 2022 by
Alexander J. Marsden,
Mark Skilbeck,
Matthew Healey,
Helen R. Thomas,
Marc Walker 
,
Rachel S. Edwards,
Natalya A. Garcia,
Filip Vuković ,
Hicham Jabraoui,
Tiffany R. Walsh ,
Jonathan P. Rourke ,
Neil R. Wilson
,
Rachel S. Edwards,
Natalya A. Garcia,
Filip Vuković ,
Hicham Jabraoui,
Tiffany R. Walsh ,
Jonathan P. Rourke ,
Neil R. Wilson
This paper is made freely available by the publisher.
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Abstract
By microscopy, spectroscopy, and modelling we show that extended topological defects are ubiquitous in oxygen functionalised graphene, whether from gas-phase or wet-chemical oxidation, and play a critical role in limiting its reduction and stiffness.