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Royal Society of Chemistry, Inorganic Chemistry Frontiers, 12(9), p. 2810-2831, 2022

DOI: 10.1039/d2qi00275b

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Large easy-axis magnetic anisotropy in a series of trigonal prismatic mononuclear cobalt(ii) complexes with zero-field hidden single-molecule magnet behaviour: the important role of the distortion of the coordination sphere and intermolecular interactions in the slow relaxation

Journal article published in 2022 by Aritz Landart-Gereka ORCID, María Mar Quesada-Moreno ORCID, Ismael F. Díaz-Ortega, Hiroyuki Nojiri ORCID, Mykhaylo Ozerov ORCID, J. Krzystek, María A. Palacios ORCID, Enrique Colacio ORCID
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

A N6-tripodal ligand allows the preparation of a family of prismatic mononuclear cationic CoII complexes with SMM behavior. Their axial anisotropy, magnetic relaxation and hysteresis width are modulated by the anion effects on the crystal structure.