Published in
Royal Society of Chemistry, Catalysis Science & Technology, 19(12), p. 5861-5868, 2022
DOI: 10.1039/d2cy01272c
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From ethene to propene (ETP) on tailored silica–alumina supports with isolated Ni(ii) sites: uncovering the importance of surface nickel aluminate sites and the carbon-pool mechanism
Journal article published in 2022 by
Zixuan Chen 
,
Scott R. Docherty ,
Pierre Florian ,
Agnieszka Kierzkowska ,
Ilia B. Moroz ,
Paula M. Abdala ,
Christophe Copéret ,
Christoph R. Müller ,
Alexey Fedorov
,
Scott R. Docherty ,
Pierre Florian ,
Agnieszka Kierzkowska ,
Ilia B. Moroz ,
Paula M. Abdala ,
Christophe Copéret ,
Christoph R. Müller ,
Alexey Fedorov
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Abstract
The ethene-to-propene reaction on Ni catalysts correlates with the formation of alkylated aromatic species. The deactivation of surface Ni aluminate sites can be reversed by calcination, while the deactivation of Ni silicate sites is irreversible.