Published in
Royal Society of Chemistry, Inorganic Chemistry Frontiers, 1(10), p. 118-126, 2023
DOI: 10.1039/d2qi01903e
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Towards panchromatic Fe(ii) NHC sensitizersviaHOMO inversion
Journal article published in 2023 by
Anil Reddy Marri 
,
Bogdan Marekha ,
Thomas Penfold ,
Stefan Haacke ,
Philippe C. Gros
,
Bogdan Marekha ,
Thomas Penfold ,
Stefan Haacke ,
Philippe C. Gros
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Abstract
Fused polythiophenes attached to Fe(ii)NHC complexes induced a mixing of the t2g and π HOMO orbitals promoting 80 nm red-shift of the MLCT transition, 3 fold increase of the molar extinction coefficient and 3MLCT excited state lifetime up to 18 ps.