Extending the π-conjugation system of covalent organic frameworks for more efficient photocatalytic H<sub>2</sub>O<sub>2</sub> production
Journal article published in 2023 by
Maojun Deng,
Jiamin Sun,
Andreas Laemont,
Chunhui Liu,
Linyang Wang,
Laurens Bourda 
,
Jeet Chakraborty,
Kristof Van Hecke ,
Rino Morent,
Nathalie De Geyter ,
Karen Leus ,
Hui Chen,
Pascal Van Der Voort
,
Jeet Chakraborty,
Kristof Van Hecke ,
Rino Morent,
Nathalie De Geyter ,
Karen Leus ,
Hui Chen,
Pascal Van Der Voort
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Abstract
Three highly crystalline and porous COFs with promising photoredox properties have been prepared. Via a post-sulfurization process, the imine-linked COFs were converted into thiazole-linked COFs, generating a highly conjugated and ultrastable photocatalyst for H2O2 production.