Published in
Royal Society of Chemistry, Catalysis Science & Technology, 4(12), p. 1289-1295, 2022
DOI: 10.1039/d1cy01807h
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A mechanistic study of syngas conversion to light olefins over OXZEO bifunctional catalysts: insights into the initial carbon–carbon bond formation on the oxide
Journal article published in 2022 by
Hongyu Chen,
Zhengmao Liu 
,
Na Li,
Feng Jiao,
Yuxiang Chen,
Zhenchao Zhao,
Meiling Guo,
Xuebin Liu,
Xiuwen Han,
Xiulian Pan ,
Xueqing Gong ,
Guangjin Hou ,
Xinhe Bao
,
Na Li,
Feng Jiao,
Yuxiang Chen,
Zhenchao Zhao,
Meiling Guo,
Xuebin Liu,
Xiuwen Han,
Xiulian Pan ,
Xueqing Gong ,
Guangjin Hou ,
Xinhe Bao
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Abstract
NMR experiments reveal a mechanism of syngas conversion in which CO reacts with OCH3 on the oxide surface, generating ketene intermediates, which can either form acetate or diffuse into zeolite.