Published in
Royal Society of Chemistry, Physical Chemistry Chemical Physics, 7(24), p. 4555-4561, 2022
DOI: 10.1039/d1cp05261f
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Interconversion between Lewis and Brønsted–Lowry acid sites on vanadia-based catalysts
Journal article published in 2022 by
Rob Jeremiah G. Nuguid 
,
Lorenzo Ortino-Ghini,
Vitaly L. Suskevich ,
Jie Yang,
Luca Lietti ,
Oliver Kröcher ,
Davide Ferri
,
Lorenzo Ortino-Ghini,
Vitaly L. Suskevich ,
Jie Yang,
Luca Lietti ,
Oliver Kröcher ,
Davide Ferri
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Abstract
Temperature, gas feed, and catalyst composition affect the interplay between Lewis acid sites (LAS) and Brønsted–Lowry acid sites (BAS). Water increases BAS not just by converting pre-existing LAS, but also by generating spontaneously new acid sites.