Published in
Royal Society of Chemistry, Physical Chemistry Chemical Physics, 9(23), p. 5496-5515, 2021
DOI: 10.1039/d0cp06267g
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Theoretical and experimental study of peroxy and alkoxy radicals in the NO<sub>3</sub>-initiated oxidation of isoprene
Journal article published in 2021 by
L. Vereecken 
,
P. T. M. Carlsson ,
A. Novelli ,
F. Bernard,
S. S. Brown ,
C. Cho ,
J. N. Crowley ,
H. Fuchs ,
W. Mellouki,
D. Reimer ,
J. Shenolikar,
R. Tillmann ,
L. Zhou,
A. Kiendler-Scharr ,
A. Wahner
,
P. T. M. Carlsson ,
A. Novelli ,
F. Bernard,
S. S. Brown ,
C. Cho ,
J. N. Crowley ,
H. Fuchs ,
W. Mellouki,
D. Reimer ,
J. Shenolikar,
R. Tillmann ,
L. Zhou,
A. Kiendler-Scharr ,
A. Wahner
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Abstract
Under atmospheric conditions, nitrate-RO2 radicals are equilibrated and react predominantly with HO2, RO2 and NO. The nitrate-RO chemistry is affected strongly by ring closure to epoxy radicals, impeding formation of MVK/MACR.