Published in
Royal Society of Chemistry, Journal of Materials Chemistry A: materials for energy and sustainability, 35(9), p. 20006-20023, 2021
DOI: 10.1039/d1ta02992d
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Energy storage mechanisms in vacancy-ordered Wadsley–Roth layered niobates
Journal article published in 2021 by
Kit McColl 
,
Kent J. Griffith ,
Rebecca L. Dally ,
Runze Li,
Jason E. Douglas,
Kenneth R. Poeppelmeier ,
Furio Corà ,
Igor Levin,
Megan M. Butala
,
Kent J. Griffith ,
Rebecca L. Dally ,
Runze Li,
Jason E. Douglas,
Kenneth R. Poeppelmeier ,
Furio Corà ,
Igor Levin,
Megan M. Butala
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Abstract
Layered niobates with vacancy-ordered Wadsley–Roth structures were investigated as Li-ion battery anodes. Using operando and ex situ methods and DFT, we identify an intercalation mechanism dominated by Li-diffusion kinetics and layer evolution.