Published in
Royal Society of Chemistry, Dalton Transactions, 14(50), p. 5011-5022, 2021
DOI: 10.1039/d1dt00881a
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Stepwise collapse of a giant pore metal–organic framework
Journal article published in 2021 by
Adam F. Sapnik 
,
Duncan N. Johnstone ,
Sean M. Collins ,
Giorgio Divitini ,
Alice M. Bumstead ,
Christopher W. Ashling ,
Philip A. Chater ,
Dean S. Keeble ,
Timothy Johnson ,
David A. Keen ,
Thomas D. Bennett
,
Duncan N. Johnstone ,
Sean M. Collins ,
Giorgio Divitini ,
Alice M. Bumstead ,
Christopher W. Ashling ,
Philip A. Chater ,
Dean S. Keeble ,
Timothy Johnson ,
David A. Keen ,
Thomas D. Bennett
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Abstract
Defect engineering is used to augment the porosity of MIL-100. Incorporation of defects leads to structural collapse and ultimately causes amorphisation. Pair distribution function analysis reveals a stepwise collapse of the hierarchical structure.