Published in
Royal Society of Chemistry, Inorganic Chemistry Frontiers, 20(7), p. 3875-3881, 2020
DOI: 10.1039/d0qi00784f
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Orientation Mapping of Rabi Frequencies in a Rare-Earth Molecular Qudit
Journal article published in 2020 by
Yu-Hui Fang 
,
Zheng Liu,
Yexin Wang,
Shen Zhou,
ShangDa Jiang ,
Song Gao
,
Zheng Liu,
Yexin Wang,
Shen Zhou,
ShangDa Jiang ,
Song Gao
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Abstract
Utilizing the S = 7/2 4f spin and the D4 symmetry of a Gd(iii) complex, we propose and demonstrate an eight-leveled rare-earth molecular qudit, which can be coherently manipulated between adjacent energy levels with precompiled pulse durations.