Published in
Royal Society of Chemistry, Journal of Materials Chemistry C Materials for optical and electronic devices, 27(8), p. 9236-9242, 2020
DOI: 10.1039/d0tc01930e
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Side-chain engineering of PEDOT derivatives as dopant-free hole-transporting materials for efficient and stable n–i–p structured perovskite solar cells
Journal article published in 2020 by
Siyuan Han,
Xiaoqing Jiang,
Ze Yu 
,
Xiaojing Wan,
Jiadong Zang,
Caiyun Zhang,
Hailong Rui,
Xichuan Yang ,
Anders Hagfeldt ,
Licheng Sun
,
Xiaojing Wan,
Jiadong Zang,
Caiyun Zhang,
Hailong Rui,
Xichuan Yang ,
Anders Hagfeldt ,
Licheng Sun
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Abstract
We report three PEDOT derivatives, namely P6, P10, and P14, by tailoring the length of the alkyl side-chains, and apply them as dopant-free HTMs in mesoscopic n–i–p structured PSCs. The devices with P10 afford the best efficiency of 16.2% together with excellent ambient stability.