Published in
Royal Society of Chemistry, Physical Chemistry Chemical Physics, 24(22), p. 13418-13430, 2020
DOI: 10.1039/c9cp07032j
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Photochemical mechanism of DEACM uncaging: A combined time-resolved spectroscopic and computational study
Journal article published in 2020 by
Carsten Hamerla,
Carsten Neumann,
Konstantin Falahati 
,
Jan von Cosel,
Luuk J. G. W. van Wilderen ,
Madhava S. Niraghatam,
Daniela Kern-Michler,
Nicole Mielke,
Matiss Reinfelds ,
Alexandre Rodrigues-Correia,
Alexander Heckel ,
Jens Bredenbeck ,
Irene Burghardt
,
Jan von Cosel,
Luuk J. G. W. van Wilderen ,
Madhava S. Niraghatam,
Daniela Kern-Michler,
Nicole Mielke,
Matiss Reinfelds ,
Alexandre Rodrigues-Correia,
Alexander Heckel ,
Jens Bredenbeck ,
Irene Burghardt
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Abstract
Combined spectroscopic and computational studies elucidate excited-state photocleavage in DEACM cages, explaining vastly different time scales for different leaving groups.