Probing the local structure of nanoscale actinide oxides: a comparison between PuO2 and ThO2 nanoparticles rules out PuO2+x hypothesis
Journal article published in 2020 by
Laura Bonato 
,
Matthieu Virot ,
Thomas Dumas ,
Adel Mesbah ,
Elodie Dalodière,
Oliver Dieste Blanco ,
Thierry Wiss ,
Xavier Le Goff ,
Michael Odorico,
Damien Prieur ,
André Rossberg,
Laurent Venault ,
Nicolas Dacheux ,
Philippe Moisy ,
Sergey I. Nikitenko
,
Matthieu Virot ,
Thomas Dumas ,
Adel Mesbah ,
Elodie Dalodière,
Oliver Dieste Blanco ,
Thierry Wiss ,
Xavier Le Goff ,
Michael Odorico,
Damien Prieur ,
André Rossberg,
Laurent Venault ,
Nicolas Dacheux ,
Philippe Moisy ,
Sergey I. Nikitenko
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Abstract
XRD, EXAFS and HR-TEM study reveals a strong correlation between AnO2 (An = Th and Pu) nanoparticle size and An(iv) local structure.