Published in
Royal Society of Chemistry, Journal of Analytical Atomic Spectrometry, 4(34), p. 636-654, 2019
DOI: 10.1039/c8ja00354h
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A unified approach to mechanistic aspects of photochemical vapor generation
Journal article published in 2019 by
Daniele Leonori 
,
Ralph E. Sturgeon
,
Ralph E. Sturgeon
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Abstract
A general model of redox reactions for PVG is proposed, driven by reducing radicals (e(aq)−, H˙, R˙ and CO2˙−) arising from concurrent VUV photolysis of carboxylic acids to yield the nascent elemental species which are subsequently attacked by H˙, H3C˙, H+and CO to yield volatile products.