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Royal Society of Chemistry, Energy & Environmental Science, 4(13), p. 1250-1258, 2020

DOI: 10.1039/c9ee03921j

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Systematic over-estimation of lattice thermal conductivity in materials with electrically-resistive grain boundaries

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

The inverse trend between carrier mobility and lattice thermal conductivity is found to be an artifact of grain boundary electrical resistance. A two-phase transport model is required to properly account for the effect.