Published in
Royal Society of Chemistry, Journal of Materials Chemistry C Materials for optical and electronic devices, 30(7), p. 9184-9194, 2019
DOI: 10.1039/c9tc02742d
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Revealing resonance effects and intramolecular dipole interactions in the positional isomers of benzonitrile-core thermally activated delayed fluorescence materials
Journal article published in 2019 by
Nadzeya A. Kukhta 
,
Heather F. Higginbotham,
Tomas Matulaitis ,
Andrew Danos ,
Aisha N. Bismillah ,
Nils Haase,
Marc K. Etherington ,
Dmitry S. Yufit ,
Paul R. McGonigal ,
Juozas Vidas Gražulevičius ,
Andrew P. Monkman
,
Heather F. Higginbotham,
Tomas Matulaitis ,
Andrew Danos ,
Aisha N. Bismillah ,
Nils Haase,
Marc K. Etherington ,
Dmitry S. Yufit ,
Paul R. McGonigal ,
Juozas Vidas Gražulevičius ,
Andrew P. Monkman
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Abstract
Rather than donor–acceptor dihedral angles, the TADF performance of DMAC–BZN positional isomers is instead controlled by differences in acceptor strength arising from π-system electron density – along with a through-space dipole interaction.