Published in
Royal Society of Chemistry, Catalysis Science & Technology, 15(9), p. 4023-4035, 2019
DOI: 10.1039/c9cy00744j
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Deactivation mechanism of hydrotalcite-derived Ni–AlOx catalysts during low-temperature CO2 methanation via Ni-hydroxide formation and the role of Fe in limiting this effect
Journal article published in 2019 by
Chalachew Mebrahtu 
,
Siglinda Perathoner ,
Gianfranco Giorgianni,
Shiming Chen ,
Gabriele Centi ,
Florian Krebs ,
Regina Palkovits ,
Salvatore Abate
,
Siglinda Perathoner ,
Gianfranco Giorgianni,
Shiming Chen ,
Gabriele Centi ,
Florian Krebs ,
Regina Palkovits ,
Salvatore Abate
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Abstract
Ni–Fe/AlOx with nanosheet structure, enhance the reducibility and stability of the Ni-hydroxide during the catalytic reaction due to the formation of spinel phase which stabilize smaller Ni nanoparticle with a weaker interaction with the support.