Published in
Royal Society of Chemistry, Physical Chemistry Chemical Physics, 5(21), p. 2283-2294, 2019
DOI: 10.1039/c8cp05950k
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Symmetry controlled excited state dynamics
Journal article published in 2019 by
Max D. J. Waters 
,
Anders B. Skov ,
Martin A. B. Larsen ,
Christian M. Clausen,
Peter M. Weber ,
Theis I. Sølling
,
Anders B. Skov ,
Martin A. B. Larsen ,
Christian M. Clausen,
Peter M. Weber ,
Theis I. Sølling
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Abstract
Symmetry effects in internal conversion are studied by means of two isomeric cyclic tertiary aliphatic amines in a velocity map imaging (VMI) experiment on the femtosecond timescale. We conclude that lessening the symmetry of the molecule leads to loss of coherence after internal conversion between Rydberg states.