Published in
Royal Society of Chemistry, Chemical Communications, 23(55), p. 3371-3374
DOI: 10.1039/c9cc00602h
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Sulfur-doped graphene for efficient electrocatalytic N2-to-NH3 fixation
Journal article published in 2019 by
Li Xia,
Jiajia Yang,
Huanbo Wang,
Runbo Zhao 
,
Hongyu Chen ,
Weihai Fang,
Abdullah M. Asiri ,
Fengyu Xie,
Ganglong Cui ,
Xuping Sun
,
Hongyu Chen ,
Weihai Fang,
Abdullah M. Asiri ,
Fengyu Xie,
Ganglong Cui ,
Xuping Sun
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Abstract
Sulfur-doped graphene (S-G) is superior for electrocatalytic ambient N2-to-NH3 fixation, offering a remarkably large NH3 yield of 27.3 μg h−1 mgcat.−1 and a high Faradaic efficiency of 11.5% at −0.6 and −0.5 V vs. a reversible hydrogen electrode, respectively, in 0.1 M HCl.