Published in
Royal Society of Chemistry, Energy & Environmental Science, 7(9), p. 2418-2432
DOI: 10.1039/c6ee01160h
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Structural and mechanistic basis for the high activity of Fe–N–C catalysts toward oxygen reduction
Journal article published in 2016 by
Jingkun Li,
Shraboni Ghoshal,
Wentao Liang,
Moulay-Tahar Sougrati 
,
Frédéric Jaouen,
Barr Halevi,
Samuel McKinney,
Geoff McCool,
Chunrong Ma,
Xianxia Yuan,
Zi-Feng Ma,
Sanjeev Mukerjee,
Qingying Jia
,
Frédéric Jaouen,
Barr Halevi,
Samuel McKinney,
Geoff McCool,
Chunrong Ma,
Xianxia Yuan,
Zi-Feng Ma,
Sanjeev Mukerjee,
Qingying Jia
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Abstract
The biomimetic dynamic nature of the Fe–N–C active site with a near-optimal Fe2+/3+redox potential facilitates ORR by balancing the site-blocking effect and O2dissociation.