Published in
Royal Society of Chemistry, Journal of Materials Chemistry A: materials for energy and sustainability, 30(6), p. 14967-14974
DOI: 10.1039/c8ta02703j
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Understanding the loss of electrochemical activity of nanosized LiMn2O4particles: a combined experimental andab initioDFT study
Journal article published in 2018 by
Ever A. Velásquez 
,
Daiane P. B. Silva,
Juliana B. Falqueto ,
José Mejía-López ,
Nerilso Bocchi ,
Rodrigo del Rio ,
Johan Mazo-Zuluaga ,
Romeu C. Rocha-Filho ,
Sonia R. Biaggio
,
Daiane P. B. Silva,
Juliana B. Falqueto ,
José Mejía-López ,
Nerilso Bocchi ,
Rodrigo del Rio ,
Johan Mazo-Zuluaga ,
Romeu C. Rocha-Filho ,
Sonia R. Biaggio
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Abstract
Nanosized spinel LMOs with crystallites smaller than ∼15 nm present significantly decreased electrochemical activity due to the increase of the energy barriers in the Li-ion diffusion paths.