Published in
Royal Society of Chemistry, Catalysis Science & Technology, 21(6), p. 7708-7717
DOI: 10.1039/c6cy00933f
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Depolymerization of 1,4-polybutadiene by metathesis: high yield of large macrocyclic oligo(butadiene)s by ligand selectivity control
Journal article published in 2016 by
Annelies Dewaele,
Tom Renders 
,
Baoyi Yu,
Francis Verpoort,
Bert F. Sels
,
Baoyi Yu,
Francis Verpoort,
Bert F. Sels
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Abstract
Herein, we demonstrate a practical high yield preparation of large macrocyclic oligo(butadiene)s, preferably the C16 to C44 fraction, from commercial 1,4-polybutadiene by exploring intramolecular backbiting using a series of commercially available Ru catalysts.