Published in

European Geosciences Union, Atmospheric Chemistry and Physics, 7(18), p. 4965-4980, 2018

DOI: 10.5194/acp-18-4965-2018

European Geosciences Union, Atmospheric Chemistry and Physics Discussions, p. 1-28

DOI: 10.5194/acp-2017-931

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Seasonal variation and chemical characterization of PM<sub>2.5</sub> in northwestern Philippines

Journal article published in 2018 by Gerry Bagtasa ORCID, Mylene G. Cayetano, Chung-Shin Yuan
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Data provided by SHERPA/RoMEO

Abstract

Abstract. The seasonal and chemical characteristics of fine particulate matter (PM2.5) were investigated in Burgos, Ilocos Norte, located at the northwestern edge of the Philippines. Each 24 h sample of fine aerosol was collected for four seasons. Fine particulate in the region shows strong seasonal variation in both concentration and composition. Highest mass concentration was seen during the boreal spring season with a mean mass concentration of 21.6 ± 6.6 µg m−3, and lowest was in fall with a mean concentration of 8.4 ± 2.3 µg m−3. Three-day wind back trajectory analysis of air mass reveals the influence of the northwestern Pacific monsoon regimes on PM2.5 concentration. During southwest monsoon, sea salt was the dominant component of fine aerosols carried by moist air from the South China Sea. During northeast monsoon, on the other hand, both wind and receptor model analysis showed that higher particulate concentration was due to the long-range transport (LRT) of anthropogenic emissions from northern East Asia. Overall, sea salt and soil comprise 33 % of total PM2.5 concentration, while local biomass burning makes up 33 %. LRT of industrial emission, solid waste burning and secondary sulfate from East Asia have a mean contribution of 34 % to the total fine particulate for the whole sampling period.