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Published in

European Geosciences Union, Atmospheric Chemistry and Physics, 11(17), p. 7055-7066, 2017

DOI: 10.5194/acp-17-7055-2017

European Geosciences Union, Atmospheric Chemistry and Physics Discussions, p. 1-14

DOI: 10.5194/acp-2017-86

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Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere

Journal article published in 2017 by Felix Ploeger, Paul Konopka ORCID, Kaley Walker ORCID, Martin Riese ORCID
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Postprint: archiving allowed
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Data provided by SHERPA/RoMEO

Abstract

Abstract. Pollution transport from the surface to the stratosphere within the Asian monsoon circulation may cause harmful effects on stratospheric chemistry and climate. Here, we investigate air mass transport from the monsoon anticyclone into the stratosphere using a Lagrangian chemistry transport model. We show how two main transport pathways from the anticyclone emerge: (i) into the tropical stratosphere (tropical pipe), and (ii) into the Northern Hemisphere (NH) extratropical lower stratosphere. Maximum anticyclone air mass fractions reach around 5 % in the tropical pipe and 15 % in the extratropical lowermost stratosphere over the course of a year. The anticyclone air mass fraction correlates well with satellite hydrogen cyanide (HCN) and carbon monoxide (CO) observations, confirming that pollution is transported deep into the tropical stratosphere from the Asian monsoon anticyclone. Cross-tropopause transport occurs in a vertical chimney, but with the pollutants transported quasi-horizontally along isentropes above the tropopause into the tropics and NH.