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Nature Research, Scientific Reports, 1(7), 2017

DOI: 10.1038/srep39844

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Model dielectric function for 2D semiconductors including substrate screening

Journal article published in 2017 by Mads Lund Trolle, Thomas Garm Pedersen ORCID, Valerie Véniard
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

AbstractDielectric screening of excitons in 2D semiconductors is known to be a highly non-local effect, which in reciprocal space translates to a strong dependence on momentum transfer q. We present an analytical model dielectric function, including the full non-linear q-dependency, which may be used as an alternative to more numerically taxing ab initio screening functions. By verifying the good agreement between excitonic optical properties calculated using our model dielectric function, and those derived from ab initio methods, we demonstrate the versatility of this approach. Our test systems include: Monolayer hBN, monolayer MoS2, and the surface exciton of a 2 × 1 reconstructed Si(111) surface. Additionally, using our model, we easily take substrate screening effects into account. Hence, we include also a systematic study of the effects of substrate media on the excitonic optical properties of MoS2 and hBN.