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Topological effects in the optical phonon dynamics of the three dimensional Dirac semimetal Cd3As2

Journal article published in 2017 by A. Sharafeev, Gnezdilov, R. Sankar, Fc C. Chou ORCID, P. Lemmens
This paper is available in a repository.
This paper is available in a repository.

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Preprint: policy unknown
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Postprint: policy unknown
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Abstract

In the three-dimensional Dirac semimetal Cd3As2 we notice an interplay of electronic and phonon degrees of freedom mediated by topological effects. There exist a pronounced quasielastic scattering and an anomalous anharmonicity of optical phonons. These effects follow a similar temperature dependence with a characteristic temperature T* ~ 100 K. Furthermore, there exist a resonant enhancement of phonon scattering intensity as function of incident photon energy. This energy of 1.9 eV coincides with interband electronic transitions in Cd3As2. A refined analysis shows that these effects are coupled via interband transitions in the Dirac states in Cd3As2 and a degeneracy of phonon energies with thermally excited electronic states. This degeneracy enhances energy density fluctuations. ; Comment: 9 pages