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Nature Research, Nature Communications, 1(8), 2017

DOI: 10.1038/ncomms15119

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Time-reversal symmetry breaking hidden order in Sr$_2$(Ir,Rh)O$_4$

Journal article published in 2017 by Jaehong Jeong ORCID, Yvan Sidis, Alex Louat, Véronique Brouet, Philippe Bourges ORCID
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Layered 5$d$ transition iridium oxides, Sr$_2$(Ir,Rh)O$_4$, are described as unconventional Mott insulators with strong spin-orbit coupling. The undoped compound, Sr$_2$IrO$_4$, is a nearly ideal two-dimensional pseudospin-$1/2$ Heisenberg antiferromagnet, similarly to the insulating parent compound of high-temperature superconducting copper oxides. Using polarized neutron diffraction, we here report a hidden magnetic order in pure and doped Sr$_2$(Ir,Rh)O$_4$, distinct from the usual antiferromagnetic pseudo-spin ordering. We find that time-reversal symmetry is broken while the lattice translation invariance is preserved in the hidden order phase. The onset temperature matches that of the odd-parity hidden order recently highlighted using optical second harmonic generation experiments. The novel magnetic order and broken symmetries can be explained by the loop-current model, previously predicted for the copper oxide superconductors. ; Comment: 7 figures: 3 in main text and 4 in the supplementary materials