European Geosciences Union, Atmospheric Chemistry and Physics, 7(17), p. 4657-4672, 2017
European Geosciences Union, Atmospheric Chemistry and Physics Discussions, p. 1-27
DOI: 10.5194/acp-2016-875
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In the frame of the SWOP (sounding water vapour, ozone, and particle) campaign during the Asian summer monsoon (ASM), ozone and water vapour profiles were measured by balloon-borne sensors launched from Lhasa (29.66° N, 91.14° E, elevation 3650 m), China, in August 2013. In total, 24 soundings were launched, nearly half of which show some strong variations in the relationship between ozone and water vapour in the tracer-tracer correlation in the upper troposphere and lower stratosphere (UTLS). 20-day backward trajectories of each sounding were calculated using the trajectory module of the Chemical Lagrangian Model of the Stratosphere (CLaMS) to analyse these variations. The trajectory calculations demonstrate that three tropical cyclones (tropical storm Jebi, typhoons Utor and Trami), which occurred over the Western Pacific Ocean during August 2013, had a considerable impact on the vertical distribution of ozone and water vapour by uplifting marine air masses to altitudes of the ASM anticyclone. Air parcels subsequently arrived at the observation site via two primary pathways: firstly via direct horizontal transport from the location of the typhoon to the station within approximately three days, and secondly via rotational subsidence, during which air parcels descend slowly along a circle following the anticyclone flow within a timescale of one week. Furthermore, the interplay between the spatial position of the ASM anticyclone and tropical cyclones plays a key role in controlling the transport pathways of air parcels from the boundary layer of the Western Pacific to Lhasa in horizontal as well as vertical transport. Moreover, the statistical analysis shows that the strongest impact by typhoons is found at altitudes between 14.5 km and 17 km (365–375 K). Low ozone values (50–80 ppbv) were observed between 370 K and 380 K due to the strong vertical transport within tropical cyclones.