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American Institute of Physics, Applied Physics Letters, 25(105), p. 253102

DOI: 10.1063/1.4904945

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Detrimental influence of catalyst seeding on the device properties of CVD-grown 2D layered materials : a case study on MoSe2

Journal article published in 2014 by M. Iqbal Bakti Utama ORCID, Xin Lu, Yanwen Yuan, Qihua Xiong
This paper was not found in any repository, but could be made available legally by the author.
This paper was not found in any repository, but could be made available legally by the author.

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Abstract

Seed catalyst such as perylene-3,4,9,10-tetracarboxylic acid tetrapotassium (PTAS) salt has been used for promoting the growth of atomically thin layered materials in chemical vapor deposition (CVD) synthesis. However, the ramifications from the usage of such catalyst are not known comprehensively. Here, we report the influence of PTAS seeding on the transistor device performance from few-layered CVD-grown molybdenum diselenide (MoSe2) flakes. While better repeatability and higher yield can be obtained with the use of PTAS seeds in synthesis, we observed that PTAS-seeded flakes contain particle impurities. Moreover, devices from PTAS-seeded MoSe2 flakes consistently displayed poorer field-effect mobility, current on-off ratio, and subthreshold swing as compared to unseeded flakes.