Abstract Longwave radiative flux divergence within the lowest 50 m of the atmospheric boundary layer was observed during the Eidgenössische Technische Hochschule (ETH) Greenland Summit experiment. The dataset collected at 72°35′N, 38°30′W, 3203 m MSL is based on longwave radiation measurements at 2 and 48 m that are corrected for the influence of the supporting tower structure. The observations cover all seasons and reveal the magnitude of longwave radiative flux divergence and its incoming and outgoing component under stable and unstable conditions. Longwave radiative flux divergence during winter corresponds to a radiative cooling of −10 K day−1, but values of −30 K day−1 can persist for several days. During summer, the mean cooling effect of longwave radiative flux divergence is small (−2 K day−1) but exhibits a strong diurnal cycle. With values ranging from −35 K day−1 around midnight to 15 K day−1 at noon, the heating rate due to longwave radiative flux divergence is of the same order of magnitude as the observed temperature tendency. However, temperature tendency and longwave radiative flux divergence are out of phase, with temperature tendency leading the longwave radiative flux divergence by 3 h. The vertical variation of the outgoing longwave flux usually dominates the net longwave flux divergence, showing a strong divergence at nighttime and a strong convergence during the day. The divergence of the incoming longwave flux plays a secondary role, showing a slight counteracting effect. Fog is frequently observed during summer nights. Under such conditions, a divergence of both incoming and outgoing fluxes leads to the strongest radiative cooling rates that are observed. Considering all data, a correlation between longwave radiative flux divergence and the temperature difference across the 2–48-m layer is found.