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American Institute of Physics, Applied Physics Letters, 20(104), p. 202409

DOI: 10.1063/1.4879456

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Epitaxial stabilization of ultra thin films of electron doped manganites

This paper is available in a repository.
This paper is available in a repository.

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Abstract

Ultra-thin films of the electron doped manganite La$_{0.8}$Ce$_{0.2}$MnO$_3$ were grown in a layer-by-layer growth mode on SrTiO$_3$ (001) substrates by pulsed laser interval deposition. High structural quality and surface morphology was confirmed by a combination of synchrotron based x-ray diffraction and atomic force microscopy. Resonant X-ray absorption spectroscopy measurements confirm the presence of Ce$^{4+}$ and Mn$^{2+}$ ions. In addition, the electron doping signature was corroborated by Hall effect measurements. All grown films show a ferromagnetic ground state as revealed by both dc magnetization and x-ray magnetic circular dichroism (XMCD) measurements and remain insulating contrary to earlier reports of a metal-insulator transition. Our results hint at the possibility of electron-hole asymmetry in the colossal magnetoresistive (CMR) manganite phase diagram akin to the high-$T_c$ cuprates.