Published in

European Geosciences Union, Atmospheric Chemistry and Physics, 1(11), p. 43-51, 2011

DOI: 10.5194/acp-11-43-2011

European Geosciences Union, Atmospheric Chemistry and Physics Discussions, 8(10), p. 18607-18633

DOI: 10.5194/acpd-10-18607-2010

Links

Tools

Export citation

Search in Google Scholar

SOSA – a new model to simulate the concentrations of organic vapours and sulphuric acid inside the ABL – Part 1: Model description and initial evaluation

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

Full text: Download

Green circle
Preprint: archiving allowed
Green circle
Postprint: archiving allowed
Green circle
Published version: archiving allowed
Data provided by SHERPA/RoMEO

Abstract

Abstract. Chemistry in the atmospheric boundary layer (ABL) is controlled by complex processes of surface fluxes, flow, turbulent transport, and chemical reactions. We present a new model SOSA (model to simulate the concentration of organic vapours and sulphuric acid) and attempt to reconstruct the emissions, transport and chemistry in the ABL in and above a vegetation canopy using tower measurements from the SMEAR II at Hyytiälä, Finland and available soundings data from neighbouring meteorological stations. Using the sounding data for upper boundary condition and nudging the model to tower measurements in the surface layer we were able to get a reasonable description of turbulence and other quantities through the ABL. As a first application of the model, we present vertical profiles of organic compounds and discuss their relation to newly formed particles.