We present rotational velocities for individual components of eleven very low mass (VLM) binaries with spectral types between M7 and L7.5. These results are based on observations taken with the near-infrared spectrograph, NIRSPEC, and the Keck II laser guide star adaptive optics (LGS AO) system. We find that the observed sources tend to be rapid rotators (vsini > 10 km/s), consistent with previous seeing-limited measurements of VLM objects. The two sources with the largest vsini, LP 349-25B and HD 130948C, are rotating at ~30% of their break up speed, and are among the most rapidly rotating VLM objects known. Furthermore, five binary systems, all with orbital semi-major axes