Published in

American Geophysical Union, Geophysical Research Letters, 5(31), p. n/a-n/a, 2004

DOI: 10.1029/2003gl018794

Links

Tools

Export citation

Search in Google Scholar

Uptake of reactive nitrogen on cirrus cloud particles during INCA: UPTAKE OF REACTIVE NITROGEN

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

Full text: Download

Green circle
Preprint: archiving allowed
Green circle
Postprint: archiving allowed
Orange circle
Published version: archiving restricted
Data provided by SHERPA/RoMEO

Abstract

The uptake of reactive nitrogen species on ice crystals in cirrus clouds was investigated by simultaneous aircraft-based measurements of gas- and condensed-phase NOy, ice particle size distribution and total aerosol surface area. The measurements were performed in 2000 during the INCA campaign at northern and southern midlatitudes at local autumn. Cirrus ice particles were frequently encountered during these flights in the upper troposphere. Concurrently with the occurrence of cirrus ice particles particulate NOy was observed. It was found that the coverage of the cirrus ice particles with particulate NOy strongly depends on the temperature and the gas-phase NOy concentration. A substantial coverage of the ice particles with values larger than one percent of a monolayer was observed only for temperatures below about 217 K. On average only about one percent of the available gas-phase NOy was found as particulate NOy.