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European Geosciences Union, Atmospheric Chemistry and Physics, 2(5), p. 461-464, 2005

DOI: 10.5194/acp-5-461-2005

European Geosciences Union, Atmospheric Chemistry and Physics Discussions, 6(4), p. 7281-7290

DOI: 10.5194/acpd-4-7281-2004

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Commentary on cloud modelling and the mass accommodation coefficient of water

Journal article published in 2005 by A. Laaksonen ORCID, T. Vesala, M. Kulmala ORCID, Pm M. Winkler, Pe E. Wagner
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Abstract. The mass accommodation coefficient of water is a quantity for which different experimental techniques have yielded conflicting values in the range 0.04-1. From the viewpoint of cloud modelling, this is an unfortunate situation, since the value of the mass accommodation coefficient affects the model results, e.g. the number concentration of activated cloud droplets. In this commentary we note that in cloud modelling, the primary quantity of interest is the droplet growth rate rather than the mass accommodation coefficient, and that experimental investigations of droplet growth rates provide more direct verification of cloud models than do measurements of the mass accommodation coefficient. Furthermore, we argue that the droplet growth rates calculated in cloud model studies are consistent with experimental results obtained so far only if a mass accommodation coefficient of unity is applied.