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CdS nanoparticle-decorated Cd nanosheets (CdS NP/Cd NSs) are successfully fabricated for the first time via a facile oxidation–sulfurization treatment of Cd nanosheets. Due to the high electrical conductivity and visible light reflectivity of Cd nanosheets, the obtained CdS NP/Cd NSs heterostructures show significantly enhanced activities for visible light-driven photocatalytic H2 production compared to other reference CdS photocatalysts.