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Wiley, Advanced Materials, 32(22), p. 3603-3607, 2010

DOI: 10.1002/adma.201000251

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Dynamic Tuning of Plasmon–Exciton Coupling in Arrays of Nanodisk–J‐aggregate Complexes

This paper is available in a repository.
This paper is available in a repository.

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Abstract

Figure Presented Dynamic tuning of plasmon-exclton resonant coupling in arrays of nanodisk-J-aggregate complexes is demonstrated. The angle-resolved spectra of an array of bare gold nanodisks exhibit continuous shifting of localized surface plasmon resonance. This characteristic enables the production of real-time, controllable spectral overlap between molecular resonance and plasmóme resonance. The resonant interaction strength as a function of spectral overlap is explored and the coupling strength changes with the incident angle of a probe light, in accord with simulations based on coupled dipóle approximation method.