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American Physical Society, Physical Review Letters, 11(109)

DOI: 10.1103/physrevlett.109.117401

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Unraveling Orbital Correlations with Magnetic Resonant Inelastic X-Ray Scattering

Journal article published in 2012 by Pasquale Marra ORCID, Krzysztof Wohlfeld, Jeroen van den Brink
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Although orbital degrees of freedom are a factor of fundamental importance in strongly correlated transition metal compounds, orbital correlations and dynamics remain very difficult to access, in particular by neutron scattering. Via a direct calculation of scattering amplitudes we show that instead magnetic resonant inelastic x-ray scattering (RIXS) does reveal orbital correlations. In contrast to neutron scattering, the intensity of the magnetic excitations in RIXS depends very sensitively on both the symmetry of the orbitals that spins occupy, and on photon polarizations. We show in detail how this effect allows magnetic RIXS to distinguish between alternating orbital ordered and ferro-orbital (or orbital liquid) states.