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Stockholm University Press, Tellus B: Chemical and Physical Meteorology, 1(61), 2009

DOI: 10.3402/tellusb.v61i1.16816

Stockholm University Press, Tellus B: Chemical and Physical Meteorology, 1(61), p. 79, 2009

DOI: 10.1111/j.1600-0889.2008.00399.x

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Spectral absorption coefficients and imaginary parts of refractive indices of Saharan dust during SAMUM-1

Journal article published in 2009 by T. Müller, A. Schladitz, A. Massling, N. Kaaden, K. Kandler ORCID, A. Wiedensohler
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

During the SAMUM-1 experiment, absorption coefficients and imaginary parts of refractive indices of mineral dust particles were investigated in southern Morocco. Main absorbing constituents of airborne samples were identified to be iron oxide and soot. Spectral absorption coefficients were measured using a spectral optical absorption photometer (SOAP) in the wavelength range from 300 to 800 nm with a resolution of 50 nm. A new method that accounts for a loading-dependent correction of fibre filter based absorption photometers, was developed. The imaginary part of the refractive index was determined using Mie calculations from 350 to 800 nm. The spectral absorption coefficient allowed a separation between dust and soot absorption. A correlation analysis showed that the dust absorption coefficient is correlated (R2 up to 0.55) with the particle number concentration for particle diameters larger than 0.5 μm, whereas the coefficient of determination R2 for smaller particles is below 0.1. Refractive indices were derived for both the total aerosol and a dust aerosol that was corrected for soot absorption. Average imaginary parts of refractive indices of the entire aerosol are 7.4 × 10−3, 3.4 × 10−3 and 2.0 × 10−3 at wavelengths of 450, 550 and 650 nm. After a correction for the soot absorption, imaginary parts of refractive indices are 5.1 × 10−3, 1.6 × 10−3 and 4.5 × 10−4.