Published in
Wiley, Angewandte Chemie International Edition, 44(52), p. 11564-11568, 2013
Wiley, Angewandte Chemie, 44(125), p. 11778-11782, 2013
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Direct Observation of Cyclic Carbenium Ions and Their Role in the Catalytic Cycle of the Methanol-to-Olefin Reaction over Chabazite Zeolites
Journal article published in 2013 by
Shutao Xu,
Anmin Zheng 
,
Yingxu Wei,
Jingrun Chen,
Jinzhe Li,
Yueying Chu,
Mozhi Zhang,
Quanyi Wang,
You Zhou,
Jinbang Wang,
Feng Deng,
Zhongmin Liu
,
Yingxu Wei,
Jingrun Chen,
Jinzhe Li,
Yueying Chu,
Mozhi Zhang,
Quanyi Wang,
You Zhou,
Jinbang Wang,
Feng Deng,
Zhongmin Liu
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Abstract
Carbenium ions in zeolites: Two important carbenium ions have been observed for the first time under working conditions of the methanol-to-olefins (MTO) reaction over chabazite zeolites using (13) C NMR spectroscopy. Their crucial roles in the MTO reaction cycles have been demonstrated by combining experiments and theoretical calculations.