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American Chemical Society, Accounts of Chemical Research, 11(40), p. 1114-1121, 2007

DOI: 10.1021/ar7000556

Wiley-VCH Verlag, ChemInform, 6(39), 2008

DOI: 10.1002/chin.200806261

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Accounting for the Unique, Doubly Dual Nature of Ionic Liquids from a Molecular Thermodynamic and Modeling Standpoint

Journal article published in 2007 by Luís Paulo N. Rebelo ORCID, Jose N. Canongia Lopes, José N. Canongia Lopes ORCID, José M. S. S. Esperança ORCID, Joanna Łachwa, Henrique J. R. Guedes, Joanna Lachwa, Vesna Najdanovic-Visak, Zoran P. Visak, Joran P. Visak
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This paper is available in a repository.

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Abstract

The fascinating, complex behavior of ionic liquids is analyzed using a molecular perspective that emphasizes the doubly dual nature of ionic liquids underlying the existence of cations and anions forming high- and low-charge-density regions. Our work bridges the liquid, gas, and solid phases spanning 5 years of research on themes as diverse as the vaporization, liquid-liquid demixing, solidification, and thermophysical behavior of ionic liquids and their mixtures and solutions.